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Orlan Arnold was an environmental chemist who conducted research on water and air pollution. Virginia Safford Arnold was a pianist and music teacher. The collection includes correspondence, professional papers, biographical material, press clippings, and photographs relating to life and careers of Orlan Arnold and Virginia Safford Arnold. Also included are genealogical and other materials for the Albright, Crawford, Safford, and Sunderland families.

The Arnold-Safford family papers contain photographic materials and mementos dating from as early as 1856, but the majority of the collection is comprised of materials from the beginning of the twentieth century through the late 1930s. The collection is divided into four series: Orlan Arnold Papers, Virginia Safford Arnold Papers, Genealogical Research, and Family Photographs and Mementos.