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Orlan Arnold was an environmental chemist who conducted research on water and air pollution. Virginia Safford Arnold was a pianist and music teacher. The collection includes correspondence, professional papers, biographical material, press clippings, and photographs relating to life and careers of Orlan Arnold and Virginia Safford Arnold. Also included are genealogical and other materials for the Albright, Crawford, Safford, and Sunderland families.

The Arnold-Safford family papers contain photographic materials and mementos dating from as early as 1856, but the majority of the collection is comprised of materials from the beginning of the twentieth century through the late 1930s. The collection is divided into four series: Orlan Arnold Papers, Virginia Safford Arnold Papers, Genealogical Research, and Family Photographs and Mementos.

The Safford Sunderland papers trace several generations of a Southeastern Michigan family, showcasing everyday life and Michigan (as well as U.S.) history over the course of the first half of the Twentieth Century.

The Safford Sunderland Family collection consists of the papers of Gertrude Sunderland Safford, her husband Homer E. Safford, his sister Ada M. Safford, and of two of the Sunderland Saffords' daughters, Helen Safford Toohy and Mildred H. Safford. The papers also contain information on and materials from Gertrude Sunderland Safford's parents, Jabez T. Sunderland and Eliza Jane Read Sunderland; her siblings, Edson Read Sunderland and Florence Sunderland; and the Sunderland Saffords' other two children, Truman Sunderland Safford and Virginia Safford Arnold. Additionally, there is some material from and on Helen Safford Toohy's husband (Clifford M. Toohy) and daughters (Janet Toohy Ferguson and Phyllis Toohy). Finally, the collection contains Ada Murray Safford's extensive genealogical materials on the Murray and Safford families.

The papers are organized into six series arranged by family member: Photographs, Gertrude Sunderland Safford, Homer Erwin Safford, Ada Murray Safford, Mildred Hortense Safford, and Helen Safford Toohy.